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Journal Articles

Research and development on membrane IS process for hydrogen production using solar heat

Myagmarjav, O.; Iwatsuki, Jin; Tanaka, Nobuyuki; Noguchi, Hiroki; Kamiji, Yu; Ioka, Ikuo; Kubo, Shinji; Nomura, Mikihiro*; Yamaki, Tetsuya*; Sawada, Shinichi*; et al.

International Journal of Hydrogen Energy, 44(35), p.19141 - 19152, 2019/07

 Times Cited Count:16 Percentile:49.6(Chemistry, Physical)

Journal Articles

R&D status in thermochemical water-splitting hydrogen production iodine-sulfur process at JAEA

Noguchi, Hiroki; Takegami, Hiroaki; Kasahara, Seiji; Tanaka, Nobuyuki; Kamiji, Yu; Iwatsuki, Jin; Aita, Hideki; Kubo, Shinji

Energy Procedia, 131, p.113 - 118, 2017/12

 Times Cited Count:22 Percentile:99.79(Energy & Fuels)

The IS process is the most deeply investigated thermochemical water-splitting hydrogen production cycle. It is in a process engineering stage in JAEA to use industrial materials for components. Important engineering tasks are verification of integrity of the total process and stability of hydrogen production in harsh environment. A test facility using corrosion-resistant materials was constructed. The hydrogen production ability was 100 L/h. Operation tests of each section were conducted to confirm basic functions of reactors and separators, etc. Then, a trial operation for integration of the sections was successfully conducted to produce hydrogen of about 10 L/h for 8 hours.

Journal Articles

IS process hydrogen production test for components and system made of industrial structural material, 2; H$$_{2}$$SO$$_{4}$$ decomposition, HI distillation, and HI decomposition section

Noguchi, Hiroki; Takegami, Hiroaki; Kamiji, Yu; Tanaka, Nobuyuki; Iwatsuki, Jin; Kasahara, Seiji; Kubo, Shinji

Proceedings of 8th International Topical Meeting on High Temperature Reactor Technology (HTR 2016) (CD-ROM), p.1029 - 1038, 2016/11

JAEA has been conducting R&D on the IS process for nuclear-powered hydrogen production. We have constructed a 100 NL/h-H$$_2$$-scale test apparatus made of industrial materials. At first, we investigated performance of components in this apparatus. In this paper, the test results of H$$_2$$SO$$_4$$ decomposition, HI distillation, and HI decomposition were shown. In the H$$_2$$SO$$_4$$ section, O$$_2$$ production rate is proportional to H$$_2$$SO$$_4$$ feed rate and SO$$_3$$ decomposition ratio was estimated about 80%. In HI distillation section, we confirmed to acquire a concentrated HI solution over azeotropic HI composition in the condenser. In HI decomposition section, H$$_2$$ could be produced stably by HI decomposer and decomposition ratio was about 18%. The H$$_2$$SO$$_4$$ decomposer, the HI distillation column, and the HI decomposer were workable. Based on the results added to that shown in Series I, we conducted a trial continuous operation and succeeded it for 8 hours.

Journal Articles

IS process hydrogen production test for components and system made of industrial structural material, 1; Bunsen and HI concentration section

Tanaka, Nobuyuki; Takegami, Hiroaki; Noguchi, Hiroki; Kamiji, Yu; Iwatsuki, Jin; Aita, Hideki; Kasahara, Seiji; Kubo, Shinji

Proceedings of 8th International Topical Meeting on High Temperature Reactor Technology (HTR 2016) (CD-ROM), p.1022 - 1028, 2016/11

Japan Atomic Energy Agency (JAEA) has manufactured 100 NL/h-H$$_2$$-scale hydrogen test apparatus. In advance to conduct the continuous operation, we investigated performance of the components in each section of the IS process. In this paper, the results of test of Bunsen and HI concentration sections was shown. In Bunsen reaction, section, we confirmed that outlet gas flow rate included no SO$$_{2}$$ gas, indicating that all the feed SO$$_{2}$$ gas was absorbed to the solution in the Bunsen reactor for the Bunsen reaction. On the basis of these results, we evaluated that Bunsen reactor was workable. In HI concentration section, HI concentration was conducted by EED stack. As a result, it can concentrate HI in HIx solution as theoretically predicted on the basis of the previous paper. Based on the results added to that shown in Series II, we have conducted a trial continuous operation and succeeded it for 8 hours.

Journal Articles

Flowsheet study of the thermochemical water-splitting IS process for effective hydrogen production

Kasahara, Seiji; Kubo, Shinji; Hino, Ryutaro; Onuki, Kaoru; Nomura, Mikihiro*; Nakao, Shinichi*

Proceedings of AIChE 2005 Spring National Meeting (CD-ROM), 8 Pages, 2005/04

Japan Atomic Energy Research Institute (JAERI) has been conducting the research and development on the thermochemical water-splitting IS process for effective hydrogen production using nuclear heat of close to 1000 $$^{circ}$$C that can be supplied from High Temperature Gas-cooled Reactor (HTGR). The activity covers the studies on the process control for the continuous hydrogen production, the process improvements in the HI decomposition procedure and the preliminary screening of corrosion resistant materials of construction. Present status of the study is presented, especially, focusing on the process flowsheeting study concerning the application of membrane process for the HI processing.

Journal Articles

Research and development of HTTR hydrogen production systems

Shiozawa, Shusaku; Ogawa, Masuro; Inagaki, Yoshiyuki; Onuki, Kaoru; Takeda, Tetsuaki; Nishihara, Tetsuo; Hayashi, Koji; Kubo, Shinji; Inaba, Yoshitomo; Ohashi, Hirofumi

Proceedings of 17th KAIF/KNS Annual Conference, p.557 - 567, 2002/04

The research and development program on nuclear production of hydrogen was started on January in 1997 as a study consigned by Ministry of Education, Culture, Sports, Science and Technology. A hydrogen production system connected to the HTTR is being designed to be able to produce hydrogen of about 4000 m3/h by steam reforming of natural gas, using a nuclear heat of 10 MW supplied by the HTTR. In order to confirm controllability, safety and performance of key components in the HTTR hydrogen production system, the facility for an out-of-pile test was constructed on the scale of approximately 1/30 of the HTTR hydrogen production system. Essential tests are also carried out to obtain detailed data for safety review and development of analytical codes. Other basic studies on the hydrogen production technology of thermochemical water splitting called an iodine sulfur (IS) process, has been carried out for more effective and various uses of nuclear heat. This paper describes the present status and a future plan on the R&D of the HTTR hydrogen production systems in JAERI.

Journal Articles

Present status of development study on HTGR heat application systems at JAERI

Higashi, Shunichi; Nakajima, Hayato; Kubo, Shinji; Onuki, Kaoru; Inagaki, Yoshiyuki; Shimizu, Saburo; Akino, Norio

Proceedings of the Seminar on HTGR Application and Development, p.164 - 175, 2001/03

no abstracts in English

Journal Articles

Preliminary process analysis for the closed cycle operation of the iodine-sulfur thermochemical hydrogen production process

*; Nakajima, Hayato; Onuki, Kaoru; Ikenoya, Kazuhiko*; Shimizu, Saburo

International Journal of Hydrogen Energy, 24(7), p.603 - 612, 1999/00

 Times Cited Count:40 Percentile:81.32(Chemistry, Physical)

no abstracts in English

Journal Articles

Screening tests on materials of construction for thermochemical IS process

Onuki, Kaoru; Ioka, Ikuo; Futakawa, Masatoshi; Nakajima, Hayato; Shimizu, Saburo; *

Zairyo To Kankyo, 46(2), p.113 - 117, 1997/00

no abstracts in English

JAEA Reports

IS Process for thermochemical hydrogen production

Onuki, Kaoru; Nakajima, Hayato; Ioka, Ikuo; Futakawa, Masatoshi; Shimizu, Saburo

JAERI-Review 94-006, 53 Pages, 1994/11

JAERI-Review-94-006.pdf:1.52MB

no abstracts in English

Journal Articles

Reaction methanol with hydriodic acid as a step of CIS process

Onuki, Kaoru; Shimizu, Saburo; Nakajima, Hayato; Ikezoe, Yasumasa; Sato, Shoichi

International Journal of Hydrogen Energy, 15(2), p.93 - 97, 1990/00

 Times Cited Count:0 Percentile:0.04(Chemistry, Physical)

no abstracts in English

Journal Articles

Laboratory scale demonstration of CIS process

Shimizu, Saburo; ; Nakajima, Hayato; Ikezoe, Yasumasa;

Int.J.Hydrogen Energy, 12(10), p.687 - 691, 1987/10

 Times Cited Count:2 Percentile:46.37(Chemistry, Physical)

no abstracts in English

Journal Articles

Studies on the nickel-iodine-sulfur process for hydrogen production, III

; Shimizu, Saburo; Nakajima, Hayato; ; Ikezoe, Yasumasa

Int.J.Hydrogen Energy, 11(9), p.571 - 575, 1986/00

 Times Cited Count:3 Percentile:60.06(Chemistry, Physical)

no abstracts in English

Journal Articles

Chemical application of nuclear reactor heat

Nihon Genshiryoku Gakkai-Shi, 27(5), p.403 - 410, 1985/00

 Times Cited Count:0 Percentile:0.02(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Studies on the nickel-iodine-sulfur process for hydrogen production, III

; Shimizu, Saburo; Nakajima, Hayato; ; Ikezoe, Yasumasa

Hydrogen Energy,Proc.5th World Conf., p.457 - 465, 1984/00

no abstracts in English

Journal Articles

Coupling of thermochemical hydrogen production processes with an HTGR

; Shimizu, Saburo; Nakajima, Hayato; Ikezoe, Yasumasa;

Int.J.Hydrogen Energy, 9(5), p.391 - 396, 1984/00

 Times Cited Count:5 Percentile:72.66(Chemistry, Physical)

no abstracts in English

Journal Articles

Studies on the nickel・iodine・sulfur process for hydrogen production

; Shimizu, Saburo; Nakajima, Hayato; ; Ikezoe, Yasumasa;

Int.J.Hydrogen Energy, 9(3), p.191 - 196, 1984/00

 Times Cited Count:6 Percentile:75.34(Chemistry, Physical)

no abstracts in English

Journal Articles

Kinetics of the thermal decomposition of nickel sulfate

; Shimizu, Saburo; Nakajima, Hayato; Ikezoe, Yasumasa;

Bulletin of the Chemical Society of Japan, 56, p.3294 - 3296, 1983/00

 Times Cited Count:2 Percentile:24.04(Chemistry, Multidisciplinary)

no abstracts in English

Journal Articles

A Nickel-iodine-sulfur process for hydrogen production

Sato, Shoichi; Shimizu, Saburo; Nakajima, Hayato; Ikezoe, Yasumasa

Int.J.Hydrogen Energy, 8(1), p.15 - 22, 1983/00

 Times Cited Count:13 Percentile:85.69(Chemistry, Physical)

no abstracts in English

JAEA Reports

Studies on Closed-Cycle Processes for Hydrogen Production V (Progress Report for the F. Y. 1980)

; Ikezoe, Yasumasa; ; Shimizu, Saburo; Nakajima, Hayato;

JAERI-M 9724, 128 Pages, 1981/10

JAERI-M-9724.pdf:3.66MB

no abstracts in English

31 (Records 1-20 displayed on this page)